clusters excited by femtosecond stimulated emission pumping

Abstract

Vibrational relaxation dynamics in I2 (Ar)n (n51,2,6,9) and I2 (CO2)n (n51,4,5) clusters are studied using femtosecond stimulated emission pumping ~fs-SEP! in conjunction with femtosecond photoelectron spectroscopy. fs-SEP generates coherently excited I2 2 within the cluster; results are reported here for excitation energies of 0.57 and 0.75 eV. The time… (More)

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