Water dynamics: dependence on local structure probed with vibrational echo correlation spectroscopy

@inproceedings{Steinel2004WaterDD,
  title={Water dynamics: dependence on local structure probed with vibrational echo correlation spectroscopy},
  author={Tobias Steinel and John B Asbury and Steven A. Corcelli and C. P. Lawrence and Jack L. Skinner and Michael D Fayer},
  year={2004}
}
Abstract Ultrafast infrared vibrational echo correlation spectroscopy with full phase information of the entire O–D stretching band of HOD in H 2 O and molecular dynamics simulations are employed to investigate water dynamics. The wavelength dependence of the measured dynamics demonstrates that different hydrogen bonded water species are subject to distinct ultrafast (∼100 fs) local fluctuations and essentially identical slower (0.4 ps to ∼2 ps) structural rearrangements. Simulations provide… CONTINUE READING

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