Vibronic and Vibrational Coherences in Two-Dimensional Electronic Spectra of Supramolecular J-Aggregates

@inproceedings{Milota2013VibronicAV,
  title={Vibronic and Vibrational Coherences in Two-Dimensional
Electronic Spectra of Supramolecular J-Aggregates},
  author={Franz Milota and Valentyn I. Prokhorenko and Tom{\'a}{\vs} Man{\vc}al and Hans von Berlepsch and Oliver Bixner and Harald Friedrich Kauffmann and J{\"u}rgen Hauer},
  booktitle={The journal of physical chemistry. A},
  year={2013}
}
In J-aggregates of cyanine dyes, closely packed molecules form mesoscopic tubes with nanometer-diameter and micrometer-length. Their efficient energy transfer pathways make them suitable candidates for artificial light harvesting systems. This great potential calls for an in-depth spectroscopic analysis of the underlying energy deactivation network and coherence dynamics. We use two-dimensional electronic spectroscopy with sub-10 fs laser pulses in combination with two-dimensional decay… CONTINUE READING
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