Two-dimensional fifth-order Raman spectroscopy of liquid formamide: Experiment and Theory.

@article{Li2008TwodimensionalFR,
  title={Two-dimensional fifth-order Raman spectroscopy of liquid formamide: Experiment and Theory.},
  author={Y L Li and L. Huang and R. J. Dwayne Miller and Tai Hasegawa and Yoshitaka Tanimura},
  journal={The Journal of chemical physics},
  year={2008},
  volume={128 23},
  pages={
          234507
        }
}
The fifth-order two-dimensional (2D) Raman spectrum of liquid formamide has been obtained. The absolute signal levels, qualitative features, as well as quantitative aspects of the 2D spectrum are found to be in good agreement with recent molecular dynamics calculations. The most important singular feature is the relatively strong rephasing signal observed along the diagonal. This finding illustrates the more structured nature of the hydrogen bond network of liquid formamide in comparison with… 
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