Surface reconstruction and chemical evolution of stoichiometric layered cathode materials for lithium-ion batteries.

Abstract

The present study sheds light on the long-standing challenges associated with high-voltage operation of LiNi(x)Mn(x)Co(1-2x)O2 cathode materials for lithium-ion batteries. Using correlated ensemble-averaged high-throughput X-ray absorption spectroscopy and spatially resolved electron microscopy and spectroscopy, here we report structural reconstruction… (More)
DOI: 10.1038/ncomms4529

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