Surface properties probed by second-harmonic and sum-frequency generation

@article{Shen1989SurfacePP,
  title={Surface properties probed by second-harmonic and sum-frequency generation},
  author={Yuen Ron Shen},
  journal={Nature},
  year={1989},
  volume={337},
  pages={519-525}
}
Optical second-harmonic generation and the related technique of infrared – visible light sum-frequency generation are extremely versatile tools for studies of many kinds of surfaces and interfaces. With the help of ultra-short laser pulses, they can be used to monitor surface dynamics and reactions with sub-picosecond time resolution. 
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