Stereogradient polymers by ruthenium-catalyzed stereospecific living radical copolymerization of two monomers with different stereospecificities and reactivities.

Abstract

Stereogradient polymers, a fundamentally new type of polymers, were prepared by the stereospecific living radical copolymerization of two monomers that have different stereospecificities and reactivities. The ruthenium-catalyzed living radical copolymerization of 2-hydroxyethyl methacrylate (HEMA) and the silyl-capped HEMA [(tert-butyldimethylsilyl)-HEMA… (More)

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