Size-resolved sea spray aerosol particles studied by vibrational sum frequency generation.

@article{Ebben2013SizeresolvedSS,
  title={Size-resolved sea spray aerosol particles studied by vibrational sum frequency generation.},
  author={Carlena J. Ebben and Andrew P Ault and Matthew J Ruppel and Olivia S Ryder and Timothy H. Bertram and Vicki H Grassian and Kimberly A. Prather and Franz M Geiger},
  journal={The journal of physical chemistry. A},
  year={2013},
  volume={117 30},
  pages={6589-601}
}
We present vibrational sum frequency generation (SFG) spectra of the external surfaces and the internal interfaces of size-selected sea spray aerosol (SSA) particles generated at the wave flume of the Scripps Hydraulics Laboratory. Our findings support SSA particle models that invoke the presence of surfactants in the topmost particle layer and indicate that the alkyl chains of surfactant-rich SSA particles are likely to be disordered. Specifically, the SFG spectra suggest that across the range… CONTINUE READING
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