Scanning Electrochemical Microscopy . 12 . Theory and Experiment of the Feedback Mode with Finite Heterogeneous Electron - Transfer Kinetics and Arbitrary Substrate Size


The theory of the feedback mode of the scanning electrochemical microscope (SECM) is extended to include the cases of both finite heterogeneous electron-transfer (et) kinetics at the substrate and arbitrary substrate sizes. Theoretical treatments are developed using two independent approaches: (i) the formulation and numerical solution of multidimensional… (More)


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