Ruddlesden-Popper Phases : Exfoliation into Sheets and Nanotubes for Assembly of Perovskite Thin Films

@inproceedings{SchaakRuddlesdenPopperP,
  title={Ruddlesden-Popper Phases : Exfoliation into Sheets and Nanotubes for Assembly of Perovskite Thin Films},
  author={Raymond E Schaak and Thomas E Mallouk}
}
Protonated Ruddlesden-Popper tantalates and titanotantalates H2[An-1BnO3n+1] (A ) Na, Ca, Sr, La; B ) Ta, Ti) that have acidic interlayer protons were exfoliated using tetra(nbutyl)ammonium hydroxide (TBA+OH-). H2CaNaTa3O10 forms both single sheets and tubular “scrolls” when reacted to make TBAxH2-xCaNaTa3O10 colloids. In contrast, TBAxH2-xA2Ta2TiO10 and TBAxH2-xALaTi2TaO10 (A ) Ca, Sr) form sheets exclusively. The n ) 2 tantalate TBAxH2-xSrTa2O7 forms high aspect ratio scrolls, as well as… CONTINUE READING

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