Real-time observation of formation and relaxation dynamics of NH4 in (CH3OH)m(NH3)n clusters.


The formation and relaxation dynamics of NH4(CH3OH)m(NH3)n clusters produced by photolysis of ammonia-methanol mixed clusters has been observed by a time-resolved pump-probe method with femtosecond pulse lasers. From the detailed analysis of the time evolutions of the protonated cluster ions, NH4(+)(CH3OH)m(NH3)n, the kinetic model has been constructed… (More)
DOI: 10.1021/jp810266a


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