Raman Measurements of Pure Hydrogen Clathrate Formation from a Supercooled Hydrogen-Water Solution.


The nucleation and growth of a solid clathrate hydrate from the liquid phase is a process that is even less understood and more difficult to study than the nucleation of a solid phase from a pure liquid. We have employed in situ Raman spectroscopy to study the hydrogen-water supercooled solution undergoing clathrate formation at a pressure of about 2 kbar… (More)
DOI: 10.1021/acs.jpclett.5b01923


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