Quantum coherence and disorder-specific effects in simulations of 2D optical spectra of one-dimensional J-aggregates.

Abstract

Time-resolved two-dimensional photon-echo (2D PE) spectra of linear J-aggregates containing four molecules per unit cell--a model system for a concentrated water solution of the pseudo-isocyanine dye--is theoretically considered. Analysis of a single unit cell and the full-sized aggregate is consistently carried out. Spectral features of a single unit cell… (More)
DOI: 10.1021/jp108291r

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