Pulse area dependence of multiple quantum coherence signals in dilute thermal gases.

@article{Ames2021PulseAD,
  title={Pulse area dependence of multiple quantum coherence signals in dilute thermal gases.},
  author={Benedikt Ames and Andreas Buchleitner and Edoardo G. Carnio and Vyacheslav N. Shatokhin},
  journal={The Journal of chemical physics},
  year={2021},
  volume={155 4},
  pages={
          044306
        }
}
In the general framework of open quantum systems, we assess the impact of the pulse area on single and double quantum coherence (1QC and 2QC) signals extracted from fluorescence emitted by dilute thermal gases. We show that 1QC and 2QC signals are periodic functions of the pulse area, with distinctive features that reflect the particles' interactions via photon exchange, the polarizations of the laser pulses, and the observation direction.Β 

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References

SHOWING 1-10 OF 59 REFERENCES
Interpreting Fluorescence Detected Two-Dimensional Electronic Spectroscopy.
Molecular Coherent Three-Quantum Two-Dimensional Fluorescence Spectroscopy.
TLDR
Molecular coherent three-quantum (3Q) two-dimensional fluorescence spectroscopy with phase cycling via shot-to-shot pulse shaping at 1 kHz repetition rate is introduced, evidencing the absence of cascades and many-particle signals of noninteracting molecules. Expand
Sensing multiple scattering via multiple quantum coherence signals
We show that multiple quantum coherence signals in dilute gases require the multiple scattering of \emph{real} photons. The latter mediate the retarded dipole-dipole interaction -- which dominates… Expand
Theory of multiple quantum coherence signals in dilute thermal gases
Manifestations of dipole-dipole interactions in dilute thermal gases are difficult to sense because of strong inhomogeneous broadening. Recent experiments reported signatures of such interactions in… Expand
Wave packet interferometry
  • 2020
Coherent multidimensional spectroscopy in the gas phase
Recent work applying multidimentional coherent electronic spectroscopy at dilute samples in the gas phase is reviewed. The development of refined phase-cycling approaches with improved sensitivity… Expand
Delocalized excitons and interaction effects in extremely dilute thermal ensembles
Long-range interparticle interactions are revealed in extremely dilute thermal atomic ensembles using highly sensitive nonlinear femtosecond spectroscopy.
Dynamical detection of dipole-dipole interactions in dilute atomic gases
  • 2019
Observation of scalable and deterministic multi-atom Dicke states in an atomic vapor
Dicke state is fundamentally responsible for many intriguing collective behaviors of many-body systems. To experimentally study how a property of multi-particle states scales with the number of… Expand
Rapid multiple-quantum three-dimensional fluorescence spectroscopy disentangles quantum pathways
TLDR
3D population-based three-dimensional electronic spectroscopy is introduced and the extraction of all fourth- and multiple sixth-order nonlinear signal contributions are extracted by employing 125-fold phase cycling of a four-pulse sequence. Expand
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