Photochemical route for accessing amorphous metal oxide materials for water oxidation catalysis.

@article{Smith2013PhotochemicalRF,
  title={Photochemical route for accessing amorphous metal oxide materials for water oxidation catalysis.},
  author={Rodney D L Smith and Mathieu S. Pr{\'e}vot and Randal D. Fagan and Zhipan Zhang and Pavel A Sedach and Man Siu and Simon Trudel and Curtis P Berlinguette},
  journal={Science},
  year={2013},
  volume={340 6128},
  pages={60-3}
}
Large-scale electrolysis of water for hydrogen generation requires better catalysts to lower the kinetic barriers associated with the oxygen evolution reaction (OER). Although most OER catalysts are based on crystalline mixed-metal oxides, high activities can also be achieved with amorphous phases. Methods for producing amorphous materials, however, are not typically amenable to mixed-metal compositions. We demonstrate that a low-temperature process, photochemical metal-organic deposition, can… CONTINUE READING
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