Optical Trapping of a Polyatomic Molecule in an ℓ-Type Parity Doublet State.
@article{Hallas2022OpticalTO, title={Optical Trapping of a Polyatomic Molecule in an ℓ-Type Parity Doublet State.}, author={Christian Hallas and Nathaniel B. Vilas and Lo{\"i}c Anderegg and Paige Robichaud and Andrew Winnicki and Chaoqun Zhang and Lan Cheng and John M. Doyle}, journal={Physical review letters}, year={2022}, volume={130 15}, pages={ 153202 } }
We report optical trapping of a polyatomic molecule, calcium monohydroxide (CaOH). CaOH molecules from a magneto-optical trap are sub-Doppler laser cooled to 20(3) μK in free space and loaded into an optical dipole trap. We attain an in-trap molecule number density of 3(1)×10^{9} cm^{-3} at a temperature of 57(8) μK. Trapped CaOH molecules are optically pumped into an excited vibrational bending mode, whose ℓ-type parity doublet structure is a potential resource for a wide range of proposed…
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