On the upconversion fluorescence in carbon nanodots and graphene quantum dots.
@article{Wen2014OnTU,
title={On the upconversion fluorescence in carbon nanodots and graphene quantum dots.},
author={Xiaoming Wen and Pyng Yu and Yon-Rui Toh and Xiaoqian Ma and Jau Tang},
journal={Chemical communications},
year={2014},
volume={50 36},
pages={
4703-6
}
}Upconversion fluorescence has been frequently cited as an important feature in carbon nanodots (CNDs) and graphene quantum dots (GQDs); and some mechanisms and potential applications have been proposed. Contrary to such a general belief, we demonstrate in this report no observable upconversion fluorescence based on five different synthesized CNDs and GQDs. We confirm that the so-called upconversion fluorescence actually originates from the normal fluorescence excited by the leaking component…
111 Citations
A misunderstanding about upconversion luminescence of carbon quantum dots
- Chemistry, PhysicsJournal of the Iranian Chemical Society
- 2014
During the recent few years, a number of articles based on detecting the upconversion luminescence in graphene quantum dots (GQDs) or carbon quantum dots (CQDs) using spectrofluorimetry with…
Carbon Quantum Dots in Nanobiotechnology
- BiologyAdvanced Structured Materials
- 2019
This chapter is expected to offer beneficial insight into the role of carbon quantum dots in biological applications and encourage more exploration on the topic.
The photoluminescence mechanism in carbon dots (graphene quantum dots, carbon nanodots, and polymer dots): current state and future perspective
- ChemistryNano Research
- 2015
At present, the actual mechanism of the photoluminescence (PL) of fluorescent carbon dots (CDs) is still an open debate among researchers. Because of the variety of CDs, it is highly important to…
Carbon Quantum Dots: Chemical Synthesis, Properties and Applications
- Chemistry, Materials Science
- 2015
Carbon quantum dots (CQDs) were accidentally discovered in 2004, and since then have attracted considerable research interest due to their unique properties and potential technological applications.…
Negative induction effect of graphite N on graphene quantum dots: tunable band gap photoluminescence
- Materials Science
- 2015
We synthesized nitrogen-doped graphene quantum dots (N-GQDs) under a high temperature range of 800–1200 °C and high pressure of 4.0 GPa through a solid-to-solid process. The graphite N in N-GQDs has…
Carbon quantum dots and their applications.
- ChemistryChemical Society reviews
- 2015
The progress in the research and development of CQDs is reviewed with an emphasis on their synthesis, functionalization and technical applications along with some discussion on challenges and perspectives in this exciting and promising field.
Glowing graphene quantum dots and carbon dots: properties, syntheses, and biological applications.
- ChemistrySmall
- 2015
The properties and synthesis methods of these carbon nanodots are reviewed and emphasis is placed on their biological (both fundamental and theranostic) applications.
Carbon quantum dots: synthesis, properties and applications
- Chemistry
- 2014
Carbon quantum dots (CQDs, C-dots or CDs), which are generally small carbon nanoparticles (less than 10 nm in size) with various unique properties, have found wide use in more and more fields during…
Facile synthesis of S, N co-doped carbon dots and investigation of their photoluminescence properties.
- ChemistryPhysical chemistry chemical physics : PCCP
- 2015
Interestingly, both down and up conversion fluorescence of the CDs show excitation-independent emission, which is quite different from most of the previously reported CDs, which provides new opportunities for fluorescence sensor designs and light energy conversion applications.
Carbon Quantum Dots: A Component of Efficient Visible Light Photocatalysts
- Chemistry
- 2017
Carbon quantum dots (CQDs) have been developed as a new member of nanocarbons, characterized by the relatively easy preparation from a wide spectrum of carbonaceous precursors through either…
References
SHOWING 1-10 OF 36 REFERENCES
Facile preparation and upconversion luminescence of graphene quantum dots.
- ChemistryChemical communications
- 2011
A facile hydrazine hydrate reduction of graphene oxide (GO) with surface-passivated by a polyethylene glycol (PEG) method for the fabrication of graphene quantum dots (GQDs) with frequency…
Synthesis and upconversion luminescence of N-doped graphene quantum dots
- Materials Science, Chemistry
- 2012
A hydrothermal approach was developed for the synthesis of N-doped graphene quantum dots (N-GQDs) by cutting N-doped graphene. The N-GQDs obtained have a N/C atomic ratio of ca. 5.6% and diameter of…
Upconversion and downconversion fluorescent graphene quantum dots: ultrasonic preparation and photocatalysis.
- Chemistry, Materials ScienceACS nano
- 2012
A facile ultrasonic route for the fabrication of graphene quantum dots (GQDs) with upconverted emission is presented, and it is interesting that the photocatalytic rate of the rutile TiO(2)/GQD complex system is ca.
Temperature-Dependent Fluorescence in Carbon Dots
- Physics
- 2012
Carbon dots are cost-effective, environmental friendly, and biocompatible nanoparticles with many potential applications in optoelectronics and biophotonics. Their dual fluorescence bands were…
Quantum-sized carbon dots for bright and colorful photoluminescence.
- Materials ScienceJournal of the American Chemical Society
- 2006
We report that nanoscale carbon particles (carbon dots) upon simple surface passivation are strongly photoluminescent in both solution and the solid state. The luminescence emission of the carbon…
Focusing on luminescent graphene quantum dots: current status and future perspectives.
- Materials ScienceNanoscale
- 2013
In this review, the state-of-the-art knowledge of GQDs is presented, with emphasis on the top-down routes which possess the advantages of abundant raw materials, large scale production and simple operation.
Carbon nanodots: synthesis, properties and applications
- Chemistry
- 2012
Carbon nanodots (C-dots) have generated enormous excitement because of their superiority in water solubility, chemical inertness, low toxicity, ease of functionalization and resistance to…
Upconversion fluorescent carbon nanodots enriched with nitrogen for light harvesting
- Chemistry
- 2012
Fluorescent nitrogen-enriched carbon nanodots (C-dots) of 1 to 3 nm were obtained through a one-pot reaction between melamine and glycerol. These C-dots show quantum yields up to 22% and a high…
Carbon dots for multiphoton bioimaging.
- Physics, ChemistryJournal of the American Chemical Society
- 2007
The two-photon luminescence microscopy imaging of human breast cancer cells with internalized carbon dots with pulsed laser excitation in the near-infrared is demonstrated.



