Observing Solvation Dynamics with Simultaneous Femtosecond X-ray Emission Spectroscopy and X-ray Scattering.

@article{Haldrup2016ObservingSD,
  title={Observing Solvation Dynamics with Simultaneous Femtosecond X-ray Emission Spectroscopy and X-ray Scattering.},
  author={Kristoffer Haldrup and Wojciech Gawelda and Rafael Abela and Roberto Alonso-Mori and Uwe Bergmann and Am{\'e}lie Bordage and Marco Cammarata and S E Canton and A O Dohn and Tim Brandt van Driel and David Mark Fritz and Andreas Galler and Pieter Glatzel and Tobias C. B. Harlang and Kasper Skov Kj{\ae}r and Henrik T Lemke and Klaus B M{\o}ller and Zolt{\'a}n N{\'e}meth and M{\'a}ty{\'a}s P{\'a}pai and Norbert S. Sas and Jens Uhlig and Diling Zhu and Gy{\"o}rgy Vank{\'o} and Villy Sundstr{\"o}m and Martin Meedom Nielsen and Christian Bressler},
  journal={The journal of physical chemistry. B},
  year={2016},
  volume={120 6},
  pages={
          1158-68
        }
}
In liquid phase chemistry dynamic solute-solvent interactions often govern the path, ultimate outcome, and efficiency of chemical reactions. These steps involve many-body movements on subpicosecond time scales and thus ultrafast structural tools capable of capturing both intramolecular electronic and structural changes, and local solvent structural changes are desired. We have studied the intra- and intermolecular dynamics of a model chromophore, aqueous [Fe(bpy)3](2+), with complementary X-ray… CONTINUE READING
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