Multidimensional femtosecond correlation spectroscopies of electronic and vibrational excitations.

@article{Mukamel2000MultidimensionalFC,
  title={Multidimensional femtosecond correlation spectroscopies of electronic and vibrational excitations.},
  author={Shaul Mukamel},
  journal={Annual review of physical chemistry},
  year={2000},
  volume={51},
  pages={
          691-729
        }
}
Femtosecond visible and infrared analogues of multiple-pulse nuclear magnetic resonance techniques provide novel snapshot probes into the structure and electronic and vibrational dynamics of complex molecular assemblies such as photosynthetic antennae, proteins, and hydrogen-bonded liquids. A classical-oscillator description of these spectroscopies in terms of interacting quasiparticles (rather than transitions among global eigenstates) is developed and sets the stage for designing new pulse… CONTINUE READING

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