Molecular structure at electrode/electrolyte solution interfaces related to electrocatalysis.


The potential dependence of the interfacial water structure at Pt and Au thin film electrodes was investigated by sum frequency generation (SFG) spectroscopy in internal reflection mode. In the case of the Pt electrode, two broad peaks were observed in the OH stretching region at ca. 3200 cm(-1) and ca. 3400 cm(-1), which are known to be due to the… (More)


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