Modulating the electronic structure of chromophores by chemical substituents for efficient energy transfer: application to fluorone.


Strong electron correlation within a quasi-spin model of chromophores was recently shown to enhance exciton energy transfer significantly. Here we investigate how the modulation of the electronic structure of the chromophores by chemical substitution can enhance energy-transfer efficiency. Unlike previous work that does not consider the direct effect of the… (More)
DOI: 10.1021/jp503900m