Lindblad equations for strongly coupled populations and coherences in photosynthetic complexes.

@article{Palmieri2009LindbladEF,
  title={Lindblad equations for strongly coupled populations and coherences in photosynthetic complexes.},
  author={Benoit Palmieri and Darius Abramavicius and Shaul Mukamel},
  journal={The Journal of chemical physics},
  year={2009},
  volume={130 20},
  pages={
          204512
        }
}
Recent experimental observations of time-resolved multidimensional signals in the light-harvesting antennae Fenna-Mathews-Olson [G. S. Engel et al., Nature (London) 446, 782 (2007)] show large oscillations of exciton populations coupled to the long-lived coherences. These effects may not be reproduced by the standard Redfield theory which assumes weak coupling to a bath. A more general relaxation superoperator which holds for all system-bath coupling parameter regimes is constructed by taking… CONTINUE READING

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Author complimentary copy. Redistribution subject to AIP license or copyright

  • Author complimentary copy. Redistribution subject to AIP license or copyright

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