Investigation of the Temperature-Induced Neutral-to-Ionic Phase Transition in the Mixed-Stack Charge-Transfer Complex TTF-CA *

Abstract

The chlorine-35 N Q R has been investigated in the mixed-stack charge-transfer complex tetrathiafluvalene-chloranil. The neutral-to-ionic (N-I) phase transit ion is clearly seen on the N Q R spectrum. Among several features of the spectra recorded and their counterpart in the sample behaviour, the evidence for the change in the crystal symmetry and the… (More)

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