Interplay of spin-orbit interactions, dimensionality, and octahedral rotations in semimetallic SrIrO(3).
@article{Nie2015InterplayOS, title={Interplay of spin-orbit interactions, dimensionality, and octahedral rotations in semimetallic SrIrO(3).}, author={Yuefeng Nie and Phil D. C. King and C. H. Kim and Masaki Uchida and H. I. Wei and Brendan D. Faeth and Jacob P. Ruf and Jacob P. C. Ruff and Lu Xie and X. Q. Pan and Craig J. Fennie and Darrell G. Schlom and Kyle M. Shen}, journal={Physical review letters}, year={2015}, volume={114 1}, pages={ 016401 } }
We employ reactive molecular-beam epitaxy to synthesize the metastable perovskite SrIrO(3) and utilize in situ angle-resolved photoemission to reveal its electronic structure as an exotic narrow-band semimetal. We discover remarkably narrow bands which originate from a confluence of strong spin-orbit interactions, dimensionality, and both in- and out-of-plane IrO(6) octahedral rotations. The partial occupation of numerous bands with strongly mixed orbital characters signals the breakdown of the…
133 Citations
Cooperative effects of lattice and spin-orbit coupling on the electronic structure of orthorhombic SrIrO₃.
- Materials ScienceJournal of physics. Condensed matter : an Institute of Physics journal
- 2015
The SOC enhanced hybridization of Ir-O orbitals serves as an explanation as to why the critical Hubbard correlation strength increases with increasing SOC strength in SrIrO3 to induce an insulating phase.
Engineering a Spin-Orbital Magnetic Insulator by Tailoring Superlattices.
- Physics, Materials SciencePhysical review letters
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Long range magnetic ordering was realized even in the m=1 single layer superlattice, implying that the design and realization of novel electronic phases is feasible at the level of a single atomic layer in complex Ir oxides.
Anisotropic magnetoresistance in spin-orbit semimetal SrIrO 3.
- Materials Science, PhysicsEuropean physical journal plus
- 2020
It is shown that the low-temperature negative magnetoresistance is anisotropic with respect to the magnetic field orientation, and its angular dependence reveals the appearance of a fourfold symmetric component above a critical magnetic field.
Monoclinic SrIrO3-a Dirac semimetal produced by non-symmorphic symmetry and spin-orbit coupling.
- Materials ScienceJournal of physics. Condensed matter : an Institute of Physics journal
- 2019
It is argued that the Dirac bands are protected by the non-symmorphic symmetry of lattice, suggesting that the semimetallic state is produced by the strong spin-orbit coupling.
Substrate-tuning of correlated spin-orbit oxides revealed by optical conductivity calculations
- PhysicsScientific reports
- 2016
Investigation of substrate-strain effects on the electronic structures of two representative Sr-iridates finds the response of the electronic structure upon tensile strain to be highly correlated with the direction of magnetic moment, the octahedral connectivity, and the SOC strength, which cooperatively determine the robustness of Jeff = 1/2 ground states.
Direct observation of the Dirac nodes lifting in semimetallic perovskite SrIrO3 thin films
- Physics, Materials ScienceScientific reports
- 2016
The data reveal that the predicted Dirac degeneracy protected by the mirror-symmetry, which was theoretically suggested to be the key to realize the non-trivial topological properties, is actually lifted in perovskite SrIrO3 thin films.
Dimensionality-driven metal-insulator transition in spin-orbit-coupled IrO2.
- PhysicsNanoscale
- 2021
A metal-insulator transition is observed in spin-orbit-coupled IrO2 thin films upon reduction of the film thickness, and magnetic measurements point to a mixed Slater- and Mott-type of insulator.
Magnetotransport of SrIrO3-based heterostructures
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Transition-metal oxide (TMO) based heterostructures provide fertile playground to explore or functionalize novel quantum materials. In this regard, the combination of 3 d and 5 d TMOs have gained…
Evidence for strong electron correlations in a nonsymmorphic Dirac semimetal
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- 2021
Metallic iridium oxides (iridates) provide a fertile playground to explore new phenomena resulting from the interplay between topological protection, spin-orbit and electron-electron interactions. To…
Slater Insulator in Iridate Perovskites with Strong Spin-Orbit Coupling.
- Physics, Materials SciencePhysical review letters
- 2016
It is reported that the substitution of nonmagnetic, isovalent Sn^4+ for Ir^{4+} in the SrIr_{1-x}Sn_{x}O_{3} perovskites synthesized under high pressure leads to a metal-insulator transition to an antiferromagnetic (AF) phase at T_{N}≥225 K.
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