Higher-order kinetic expansion of quantum dissipative dynamics: mapping quantum networks to kinetic networks.

@article{Wu2013HigherorderKE,
  title={Higher-order kinetic expansion of quantum dissipative dynamics: mapping quantum networks to kinetic networks.},
  author={Jianlan Wu and Jianshu Cao},
  journal={The Journal of chemical physics},
  year={2013},
  volume={139 4},
  pages={
          044102
        }
}
We apply a new formalism to derive the higher-order quantum kinetic expansion (QKE) for studying dissipative dynamics in a general quantum network coupled with an arbitrary thermal bath. The dynamics of system population is described by a time-convoluted kinetic equation, where the time-nonlocal rate kernel is systematically expanded of the order of off-diagonal elements of the system Hamiltonian. In the second order, the rate kernel recovers the expression of the noninteracting-blip… CONTINUE READING

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