Frequency dependence of specific heat in supercooled liquid water and emergence of correlated dynamics.

@article{Saito2013FrequencyDO,
  title={Frequency dependence of specific heat in supercooled liquid water and emergence of correlated dynamics.},
  author={Shinji Saito and Iwao Ohmine and Biman Bagchi},
  journal={The Journal of chemical physics},
  year={2013},
  volume={138 9},
  pages={
          094503
        }
}
Molecular origin of the well-known specific heat anomaly in supercooled liquid water is investigated here by using extensive computer simulations and theoretical analyses. A rather sharp increase in the values of isobaric specific heat with lowering temperature and the weak temperature dependence of isochoric specific heat in the same range are reproduced in simulations. We calculated the spatio-temporal correlation among temperature fluctuations and examined the frequency dependent specific… 

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