Fluorescence correlation spectroscopy as a tool to investigate single molecule probe dynamics in thin polymer films.

@article{Casoli2001FluorescenceCS,
  title={Fluorescence correlation spectroscopy as a tool to investigate single molecule probe dynamics in thin polymer films.},
  author={A Casoli and Monika Sch{\"o}nhoff},
  journal={Biological chemistry},
  year={2001},
  volume={382 3},
  pages={363-9}
}
Fluorescence correlation experiments were performed on rhodamine 6G in PDMS spin-coated films on glass surfaces. With polarised excitation, ensemble bleaching of the dye and single molecule intensity fluctuations were observed. From the statistics of single molecule intensity data taken at different positions in the film, correlation functions were calculated. Two modes of motion with exponential decay shapes and correlation times of tau(c) = 0.15 s and tau(c) = 0.7 s could be detected… CONTINUE READING
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References

Publications referenced by this paper.
Showing 1-10 of 21 references

Correlation spectroscopy of individual molecules immobilized on surfaces under ambient conditions

  • C. Tietz, R. Daum, +5 authors von Borczyskowski
  • Chem. Phys. Lett. 282, 164 – 170.
  • 1998
Highly Influential
5 Excerpts

Room-temperature fluorescence characteristics of single dye molecules adsorbed on a glass surface

  • K. D. Weston, P. J. Carson, H. Metiu, S. K. Buratto
  • J. Chem. Phys. 109, 7474 – 7485.
  • 1998
Highly Influential
3 Excerpts

Emission of the contact ion pair of rhodamine dyes observed by single molecule spectroscopy

  • F. Köhn, J. Hofkens, F. C. de Schryver
  • Chem. Phys. Lett. 321, 372 – 378.
  • 2000
2 Excerpts

Ten years of single-molecule spectroscopy

  • P. Tamarat, A. Maali, B. Lounis, M. Orrit
  • J. Phys. Chem. A 104, 1 – 16.
  • 2000
2 Excerpts

Polarizations spectroscopy of single fluorescent molecules

  • T. Ha, T. A. Laurence, D. S. Chemla, S. Weiss
  • J. Phys. Chem. B 103, 6839– 6850.
  • 1999
1 Excerpt

Single Molecules as Probes of Lipid Membrane Microenvironments

  • C. E. Talley, R. C. Dunn
  • J. Phys. B 103, 10214 – 10220.
  • 1999
2 Excerpts

larizations spectroscopy of single fluorescent molecules

  • T. Ha, T. A. Laurence, D. S. Chemla, S. Weiss
  • J . Phys . Chem . B
  • 1999
1 Excerpt

Fluorescence intensity fluctuations of single atoms, molecules and nanoparticles

  • T. Basché
  • J. Lumin. 76/77, 263 – 269.
  • 1998
2 Excerpts

Microheterogeneity in dye-doped silicate and polymer films

  • H. Wang, A. M. Bardo, M. M. Collison, D. A. Higgins
  • J. Phys. Chem. B 102, 7231 – 7237.
  • 1998
2 Excerpts

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