Femtosecond dynamics of dative bonding: concepts of reversible and dissociative electron transfer reactions.


With fs time, speed, and angular resolution of the elementary steps in electron transfer reactions, we report direct observation of reversible and dissociative processes for dative bonding involving covalent and ionic characters. For bimolecular reactions of various donors and acceptors we find strong correlation between the structure and the dynamics. The… (More)


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