Femtosecond broadband stimulated Raman spectroscopy: Apparatus and methods.

  title={Femtosecond broadband stimulated Raman spectroscopy: Apparatus and methods.},
  author={David W McCamant and Philipp Kukura and Sangwoon Yoon and Richard A Mathies},
  journal={The Review of scientific instruments},
  volume={75 11},
The laser, detection system, and methods that enable femtosecond broadband stimulated Raman spectroscopy (FSRS) are presented in detail. FSRS is a unique tool for obtaining high time resolution (<100 fs) vibrational spectra with an instrument response limited frequency resolution of <10 cm(-1). A titanium:Sapphire-based laser system produces the three different pulses needed for FSRS: (1) A femtosecond visible actinic pump that initiates the photochemistry, (2) a narrow bandwidth picosecond… CONTINUE READING
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