Elucidating the Nature of the Excited State of a Heteroleptic Copper Photosensitizer by using Time-Resolved X-ray Absorption Spectroscopy.

Abstract

We report the light-induced electronic and geometric changes taking place within a heteroleptic CuI photosensitizer, namely [(xant)Cu(Me2 phenPh2 )]PF6 (xant=xantphos, Me2 phenPh2 =bathocuproine), by time-resolved X-ray absorption spectroscopy in the ps-μs time regime. Time-resolved X-ray absorption near edge structure (XANES) and extended X-ray absorption… (More)
DOI: 10.1002/chem.201800330

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