Electrochemical Stimuli-Driven Facile Metal-Free Hydrogen Evolution from Pyrene-Porphyrin-Based Crystalline Covalent Organic Framework.

@article{Bhunia2017ElectrochemicalSF,
  title={Electrochemical Stimuli-Driven Facile Metal-Free Hydrogen Evolution from Pyrene-Porphyrin-Based Crystalline Covalent Organic Framework.},
  author={Subhajit Bhunia and S. Das and Rajkumar Jana and S. C. Peter and Santanu Bhattacharya and M. Addicoat and A. Bhaumik and A. Pradhan},
  journal={ACS applied materials \& interfaces},
  year={2017},
  volume={9 28},
  pages={
          23843-23851
        }
}
A [2 + 2] Schiff base type condensation between 5,10,15,20-tetrakis(4-aminophenyl)porphyrin (TAP) and 1,3,6,8-tetrakis (4-formylphenyl) pyrene (TFFPy) under solvothermal condition yields a crystalline, quasi-two-dimensional covalent organic framework (SB-PORPy-COF). The porphyrin and pyrene units are alternatively occupied in the vertex of 3D triclinic crystal having permanent microporosity with moderately high surface area (∼869 m2 g-1) and promising chemical stability. The AA stacking of the… Expand
Iron-porphyrin-based covalent-organic frameworks for electrochemical sensing H2O2 and pH.
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