Effect of the potential well on vibrational scattering and the validity of SSH theory


The vibrational de-excitation probability, P 10, is calculated quantum mechanically over a large energy range for models of three collision systems: 0 2-02, Cl2-Cl2, and Br2-Br2• The vibrational de-excitation cross section, <r 1ao is similarly calculated for the Cl2-Cl2 model. P 10 and <r 10 are obtained for the Lennard-Jones intermolecular potential and… (More)

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