Communication: Probing the interaction of infrared antenna arrays and molecular films with ultrafast quantum dynamics.


Narrowband vibrational molecular transitions interacting with the broadband resonance of infrared plasmonic antennas lead to Fano lineshapes observed in linear (FTIR) and third-order (transient absorption and 2DIR) spectroscopic experiments. Both molecular and plasmonic components are inherently dissipative, and the effects associated with their coupling… (More)
DOI: 10.1063/1.5025600


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