Coherent control of indirect photofragmentation in the weak-field limit: control of transient fragment distributions.


We demonstrate theoretically that laser-induced coherent quantum interference control of asymptotic states of dissociating molecules is possible--even in the (one-photon) weak-field limit starting from a single vibrational eigenstate--when resonances are in play. This is illustrated for the NaI molecule, where it is shown that the probability of observing… (More)
DOI: 10.1063/1.3582928


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