Artificial chemotaxis of phoretic swimmers: instantaneous and long-time behaviour
@article{TtuleaCodrean2018ArtificialCO, title={Artificial chemotaxis of phoretic swimmers: instantaneous and long-time behaviour}, author={Maria Tătulea-Codrean and Eric Lauga}, journal={Journal of Fluid Mechanics}, year={2018}, volume={856}, pages={921 - 957} }
Phoretic swimmers are a class of artificial active particles that has received significant attention in recent years. By making use of self-generated gradients (e.g. in temperature, electric potential or some chemical product) phoretic swimmers are capable of self-propulsion without the complications of mobile body parts or a controlled external field. Focusing on diffusiophoresis, we quantify in this paper the mechanisms through which phoretic particles may achieve chemotaxis, both at the…
19 Citations
Phoretic and hydrodynamic interactions of weakly confined autophoretic particles.
- 2019
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The Journal of chemical physics
This work proposes a first model for the interaction of phoretic particles in Hele-Shaw confinement and shows that in this limit, hydrodynamic and phoretIC interactions share not only the same scaling but also the same form, albeit in opposite directions.
Hydrochemical interactions in dilute phoretic suspensions: From individual particle properties to collective organization
- 2020
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Physical Review Fluids
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Modeling chemo-hydrodynamic interactions of phoretic particles: A unified framework
- 2019
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Physical Review Fluids
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Active fluids - Interactions and collective dynamics in phoretic suspensions
- 2019
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- 2021
Biology
Scientific Reports
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Hydrochemical interactions of phoretic particles: a regularized multipole framework
- 2021
Computer Science
Journal of Fluid Mechanics
This work proposes a regularized multipole framework, directly inspired by the force coupling method (FCM), to model phoretic suspensions, and relies on grid-based volume averages of the concentration field to compute the particle surface concentration moments.
Stochastic dynamics of dissolving active particles
- 2019
Mathematics
The European physical journal. E, Soft matter
This work develops and compares two distinct chemical models for the decay of a swimmer, taking into account the material composition and nature of the chemical or enzymatic reaction at its surface, and investigates mathematically the dynamics of degradable active particles.
Estimating the velocity of chemically-driven Janus colloids considering the anisotropic concentration field
- 2022
Physics
Frontiers in Chemistry
The application of the active colloids is strongly related to their self-propulsion velocity, which is controlled by the generated anisotropic concentration field. We investigated the effect of this…
Autophoresis of two adsorbing/desorbing particles in an electrolyte solution
- 2019
Physics
Journal of Fluid Mechanics
Classical diffusiophoresis describes the motion of particles in an electrolyte or non-electrolyte solution with an imposed concentration gradient. We investigate the autophoresis of two particles in…
Active Janus colloids at chemically structured surfaces.
- 2019
Chemistry
The Journal of chemical physics
This study uses a point-particle approximation combined with a multipole expansion in order to discuss the effects of pattern geometry and chemical contrast on the particle trajectories, and considers planar walls patterned with chemical steps and stripes.
53 References
Dynamics and efficiency of a self-propelled, diffusiophoretic swimmer.
- 2012
Environmental Science
The Journal of chemical physics
This work considers several aspects relating to the dynamics of the swimming particle and employs irreversible, linear thermodynamics to formulate an energy balance, highlighting the importance of solute convection for a consistent treatment of the energetics.
Phoretic self-propulsion at finite Péclet numbers
- 2014
Physics
Journal of Fluid Mechanics
Abstract Phoretic self-propulsion is a unique example of force- and torque-free motion on small scales. The classical framework describing the flow field around a particle swimming by…
Chemotaxis of artificial microswimmers in active density waves.
- 2016
Biology
Physical review. E
This work investigates the transport of artificial swimmers subject to traveling active waves and shows, by means of analytical and numerical methods, that self-propelled particles can actually diffuse in either direction with respect to the wave, depending on its speed and waveform.
Clusters, asters, and collective oscillations in chemotactic colloids.
- 2014
Biology
Physical review. E, Statistical, nonlinear, and soft matter physics
This work presents a comprehensive theoretical description of gradient-sensing of an individual swimmer, leading controllably to chemotactic or anti-chemotactic behavior, and uses it to construct a framework for studying their collective behavior.
Phoretic motion of spheroidal particles due to self-generated solute gradients
- 2010
Physics
The European physical journal. E, Soft matter
This work derives an analytical expression for the phoretic velocity of a spheroidal particle, which generates solute gradients in the surrounding unbounded solvent via chemical reactions active on its surface in a cap-like region centered at one of the poles of the particle.
Designing phoretic micro- and nano-swimmers
- 2007
Environmental Science
Small objects can swim by generating around them fields or gradients which in turn induce fluid motion past their surface by phoretic surface effects. We quantify for arbitrary swimmer shapes and…
Taylor dispersion of gyrotactic swimming micro-organisms in a linear flow
- 2002
Physics
The theory of generalized Taylor dispersion for suspensions of Brownian particles is developed to study the dispersion of gyrotactic swimming micro-organisms in a linear shear flow. Such creatures…
Dynamic clustering and chemotactic collapse of self-phoretic active particles.
- 2014
Physics
Physical review letters
This work identifies two dynamic clustering states and characterize them by power-law-exponential distributions and predicts that in case of mere attraction a chemotactic collapse occurs directly from the gaslike into the collapsed state, which it also predicts by mapping the Langevin dynamics on the Keller-Segel model for bacterial chemotaxis.
The hydrodynamics of swimming microorganisms
- 2009
Biology, Engineering
The biophysical and mechanical principles of locomotion at the small scales relevant to cell swimming, tens of micrometers and below are reviewed, with emphasis on the simple physical picture and fundamental flow physics phenomena in this regime.
Biased swimming cells do not disperse in pipes as tracers: A population model based on microscale behaviour
- 2012
Engineering, Biology
A Galerkin method is presented to calculate the local mean swimming velocity and diffusion tensor based on local shear for arbitrary flow rates and is validated with asymptotic results obtained in the limits of weak and strong shear.