A Continuum of Proton-Coupled Electron Transfer Reactivity.

@article{Darcy2018ACO,
  title={A Continuum of Proton-Coupled Electron Transfer Reactivity.},
  author={Julia W Darcy and Brian M. Koronkiewicz and Giovanny A Parada and James M Mayer},
  journal={Accounts of chemical research},
  year={2018},
  volume={51 10},
  pages={
          2391-2399
        }
}
Proton-coupled electron transfer (PCET) covers a wide range of reactions involving the transfer(s) of electrons and protons. The best-known PCET reaction, hydrogen atom transfer (HAT), has been studied in detail for more than a century. HAT is generally described as the concerted transfer of a hydrogen atom (H• ≡ H+ + e-) from one group to another, Y + H-X → Y-H + X, but a strict definition of HAT has been difficult to establish. Distinctions are more challenging when the transfer of "H… CONTINUE READING
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