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Solar-driven reforming of lignocellulose to H 2 with a CdS/CdO x photocatalyst
This work was supported by the Christian Doppler Research Association (Austrian Federal Ministry of Science, Research and Economy and the National Foundation for Research, Technology and…
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Tuning Product Selectivity for Aqueous CO2 Reduction with a Mn(bipyridine)-pyrene Catalyst Immobilized on a Carbon Nanotube Electrode
TLDR
The assembly of a [MnBr(2,2′-bipyridine)(CO)3] complex anchored to a carbon nanotube electrode via a pyrene unit is reported, emphasizing the advantages of integrating molecular catalysts onto electrode surfaces for enhancing catalytic activity while allowing excellent control and a deeper understanding of the catalytic mechanisms.
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Multihole water oxidation catalysis on haematite photoanodes revealed by operando spectroelectrochemistry and DFT
TLDR
Spectroelectrochemical evidence together with density functional theory calculations show that charge accumulation determines the reaction mechanism on metal–oxide photoanodes, and features that are common to the mechanisms of water oxidation carried out by other inorganic and biological systems are revealed.
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Pathways to electrochemical solar-hydrogen technologies
Solar-powered electrochemical production of hydrogen through water electrolysis is an active and important research endeavor. However, technologies and roadmaps for implementation of this process do…
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Electrocatalytic and Solar‐Driven CO2 Reduction to CO with a Molecular Manganese Catalyst Immobilized on Mesoporous TiO2
TLDR
UV/vis spectroscopy confirmed that an active Mn–Mn dimer was formed during catalysis on the TiO2 electrode, showing the dynamic formation of a catalytically active dimer on an electrode surface.
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Understanding Immobilized Molecular Catalysts for Fuel-Forming Reactions through UV/Vis Spectroelectrochemistry
Molecular catalysis of fuel-forming half reactions such as proton and CO2 reduction is a key area of study for achieving electrical-to-chemical energy storage and solar fuel synthesis. Immobilization…
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Energy transfer and photoluminescence properties of lanthanide-containing polyoxotitanate cages coordinated by salicylate ligands.
TLDR
An energy-transfer mechanism involving the salicylate-to-Ti4+ charge-transfer state is proposed to account for the largely red-shifted excitation wavelengths of these Ln-1 cages, among the highest reported values for Nd3+-complexes in the literature.
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Precious-metal free photoelectrochemical water splitting with immobilised molecular Ni and Fe redox catalysts
Splitting water into hydrogen and oxygen with 3d transition metal molecular catalysts and light has been accomplished.
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Enhanced oxygen evolution catalysis by aluminium-doped cobalt phosphide through in situ surface area increase
The deployment of water electrolysis as a major contributor to global hydrogen production requires the elimination of catalysts based on scarce and expensive precious metals, and amongst the most…
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Asymmetric synthesis of syn- and anti-a-deuterio- 3-phenylalanine derivatives
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