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Abstract Intact natural gas hydrate of structure II made up more than 80% of the water present in nearbottom core material recovered from the Gulf of Mexico. Solid-state carbon-13 nuclear magnetic… (More)
Since the mid-1950s it has been known that most simple clathrate hydrates belong to one of two cubic crystal forms known as type I and II1–3. Only recently it was established that structure II… (More)
X-ray and neutron diffraction studies show argon and krypton to preferentially form clathrate hydrates of structure II, rather than structure I as previously assumed; methane and hydrogen sulphide do… (More)