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Cross-phase modulation (XPM) and induced focusing occur when copropagating ultrafast pulses interact in a nonlinear medium. XPM and induced focusing are investigated as new techniques to control the spectral, temporal, and spatial properties of ultrafast pulses with femtosecond time response. In this paper we review our most recent measurements on (1)… (More)
Archimedes micro-screws have been fabricated by three-dimensional two-photon polymerization using a Nd:YAG Q-switched microchip laser at 532nm. Due to their small sizes they can be easily manipulated, and made to rotate using low power optical tweezers. Rotation rates up to 40 Hz are obtained with a laser power of 200 mW, i.e. 0.2 Hz/mW. A photo-driven… (More)
This study proposes an optically driven complex micromachine with an Archimedes microscrew as the mechanical power, a sphere as a coupler, and three knives as the mechanical tools. The micromachine is fabricated by two-photon polymerization and is portably driven by optical tweezers. Because the microscrew can be optically trapped and rotates spontaneously,… (More)
We report here the synthesis and characterization of a new type of non-ionic blue fluorescent water-soluble chromophores specifically designed for two-photon absorption microscopy. The water solubility is induced by introduction of short oligo(ethylene glycol) monomethyl ether moieties. This work has led to low molecular weight dyes with efficient… (More)
In this study, we characterized the rotational efficiency of the photo-driven Archimedes screw. The micron-sized Archimedes screws were fabricated using the two-photon polymerization technique. Free-floating screws trapped by optical tweezers align in the laser irradiation direction and rotate spontaneously. The influences of the screw pitch and the number… (More)
A molecular engineering strategy based on rational variations of the bromine substitution pattern in two-photon absorbing singlet oxygen sensitizers allows studying the relations that exist between the positioning of an inter-system crossing promoter on the charge-transfer chromophore and its ability to generate singlet oxygen.
The design of new chromophores presenting simultaneous SHG and TPEF properties is reported.
(3) Synthesis and characterizations of the RuL1TEG complex p. 6 (3) Spectroscopic measurements p. 8 (4) Tissue culture conditions p. 9 (5) Drug and light exposure conditions p. 10 (6) Figure S1 : UV/Vis absorption spectrum and emission spectrum of the RuL1PEG complex p. 11 (7) Figure S2 : Fluorescence image of F98 cells loaded with the RuL1TEG complex.… (More)
Two europium complexes with bis(bipyridine) azamacrocyclic ligands featuring pendant arms with or without π-conjugated donor groups are synthesized and fully characterized by theoretical calculations and NMR spectroscopy. Their photophysical properties, including two-photon absorption, are investigated in water and in various organic solvents. The… (More)