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Abstract Compounds 7–8 , monoterpenic analogues of the marine metabolites puupehenone ( 1 ) and puupehedione ( 2 ), were prepared from the easily available β-cyclocitral ( 10 ) and the aryllithium… (More)
The titanocene-catalyzed cascade cyclization of epoxypolyenes, which are easily prepared from commercially available polyprenoids, has proven to be a useful procedure for the synthesis of C(10),… (More)
A new route to podolactones functionalized in the A ring has been achieved. Two key steps were employed in this synthesis, the construction of the bicyclic skeleton via a Mn(III)-mediated radical… (More)
The cationic cyclization of polyenes has proved to be a useful tool in the synthesis of natural terpenic products.1 During recent years biomimetic approaches using radical chemistry have also been… (More)