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In a molecular triad comprised of a central naphthalene diimide (NDI) unit flanked by two [Ru(bpy)3]2+ (bpy = 2,2'-bipyridine) sensitizers, NDI2- is formed after irradiation with visible light in deaerated CH3CN in the presence of excess triethylamine. The mechanism for this electron accumulation involves a combination of photoinduced and thermal elementary… (More)