Jeffrey W Beattie

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Herein we describe bimetallic di-nickel and di-copper complexes [Ni2(L)Br4] (1) and [Cu2(L)Br4(NCMe)2] (2) (L = (1E,1'E)-N,N'-(1,4-phenylenebis(methylene))bis(1-(6-(2,4,6-triisopropylphenyl)pyridin-2-yl)methanimine)) that bind oxalate intramolecularly to form [Ni2(L)Br2(C2O4)(NCMe)] (3) and [Cu2(L)Br2(C2O4)] (4). For the di-nickel complex 1, oxalate(More)
The dinuclear complex Ni(2)L(1)(η(2)-CS(2))(2) (2), featuring iminopyridine ligation, is prepared by COD substitution from Ni(2)L(1)(COD)(2) (1). Spectroscopic, structural, and theoretical data reveals significant activation of the metal-bound C-S bonds, as well as the different oxidation states of the iminopyridine in (1-) and (0).
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