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Many of the models used for the assessment of the potential risk from a radioactive waste repository require an input of data relating to the solubility of a large number of radionuclides. The Nirex… (More)
Abstract The solubilities of thorium, protactinium, uranium, neptunium, plutonium, and americium under the chemical conditions representative of a cementitious near-field environment have been… (More)
Abstract When uranium or plutonium undergoes fission, the mean valency of the resulting fission product mixture may differ from that of the starting material. This paper describes the use of a… (More)
The results of an experimental study of the sorption of uranium onto clay at pH 8 and pH 11 have been successfully simulated using a triple layer sorption model. The model has been incorporated in a… (More)
Abstract Four miniature fuel pins containing uranium/plutonium oxide, covering a wide range of oxygen-to-metal ratios, have been irradiated in a thermal reactor. These pins were subjected to a… (More)
The solubility of some of the radiologically important actinide elements have been determined in a water whose chemistry was representative of that believed to exist in potential repositories in the… (More)