Daniel R Fandrick

Publications79
h-index20
Citations1,341
Highly Influential Citations1
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N-Heterocyclic Carbene-Catalyzed Silyl Enol Ether Formation.
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The Growing Impact of Catalysis in the Pharmaceutical Industry
Catalysis has become increasingly important for the pharmaceutical industry. Catalysis is a critical technology that enables economical and environmentally-sound manufacturing processes. The… Expand
  • 269
Copper catalyzed asymmetric propargylation of aldehydes.
The highly enantio- and regioselective copper catalyzed asymmetric propargylation of aldehydes with a propargyl borolane reagent is reported. The methodology demonstrated broad functional group… Expand
  • 77
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Dynamic kinetic asymmetric cycloadditions of isocyanates to vinylaziridines.
The first examples of the use of racemic vinylaziridines in a Pd-catalyzed dynamic kinetic asymmetric transformation have been examined. Optimization studies of the Pd-catalyzed addition of… Expand
  • 87
Room temperature palladium-catalyzed cross coupling of aryltrimethylammonium triflates with aryl Grignard reagents.
Aryltrimethylammonium triflates and tetrafluoroborates were found to be highly reactive electrophiles in the Pd-catalyzed cross coupling with aryl Grignard reagents. The coupling reactions proceed at… Expand
  • 88
Dynamic kinetic asymmetric allylic alkylations of allenes.
The dynamic kinetic asymmetric allylic alkylations of racemic allene acetates has been developed with the DACH−phenyl Trost ligand 2 to give general access to allenes with high enantiomeric excess… Expand
  • 83
A general copper-BINAP-catalyzed asymmetric propargylation of ketones with propargyl boronates.
An operationally simple copper-BINAP-catalyzed, highly enantioselective propargylation of ketones is presented. The methodology was developed as an enantioselective process for methyl ethyl ketone… Expand
  • 46
Dynamic kinetic asymmetric allylic amination and acyl migration of vinyl aziridines with imido carboxylates.
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DYKAT of vinyl aziridines: total synthesis of (+)-pseudodistomin D.
A concise total synthesis of (+)-pseudodistomin D was developed. The absolute stereochemistry was established through a dynamic kinetic asymmetric cycloaddition of an isocyanate to a vinyl aziridine.… Expand
  • 61
Zinc-catalyzed allenylations of aldehydes and ketones.
The general zinc-catalyzed allenylation of aldehydes and ketones with an allenyl boronate is presented. Preliminary mechanistic studies support a kinetically controlled process wherein, after a… Expand
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