Daigo Miyajima

Publications38
h-index15
Citations1,479
Highly Influential Citations5
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A rational strategy for the realization of chain-growth supramolecular polymerization
TLDR
The realization of chain-growth polymerization is reported by designing metastable monomers with a shape-promoted intramolecular hydrogen-bonding network that enables optical resolution of a racemic monomer.
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An autonomous actuator driven by fluctuations in ambient humidity.
TLDR
An unprecedented film actuator that seemingly operates autonomously is reported, because it responds to the adsorption and desorption of a minute amount of water, possibly induced by fluctuations in the ambient humidity.
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Cyclic block copolymers for controlling feature sizes in block copolymer lithography.
TLDR
This study demonstrates that macromolecular architecture is also a powerful tool for tuning domain spacing, and a new synthetic strategy for cyclic block polymers based on highly efficient "click" coupling of difunctional linear chains is developed.
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Revisiting thiol‐yne chemistry: Selective and efficient monoaddition for block and graft copolymer formation
The untapped potential of radical thiol-yne mono-addition chemistry is exploited to overcome the known limitations of thiol-ene chemistry in polymer coupling and block copolymer formation. By careful…
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Ferroelectric Columnar Liquid Crystal Featuring Confined Polar Groups Within Core–Shell Architecture
TLDR
A ferroelectric response is reported for a columnar liquid crystal adopting a core–shell architecture that accommodates an array of polar cyano groups confined by a hydrogen-bonded amide network with an optimal strength.
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Liquid crystalline corannulene responsive to electric field.
TLDR
An amide-appended corannulene derivative with tribranched paraffinic side chains self-assembles into a hexagonal columnar liquid crystalline (LC) mesophase that responds to an applied electric field and can align homeotropically to the electrode surface.
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Thermally bisignate supramolecular polymerization.
TLDR
A supramolecular polymerization that occurs upon heating as well as cooling is reported, which may lead to supramolescular polymers with tailored complex thermoresponsive properties.
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Columnar liquid crystal with a spontaneous polarization along the columnar axis.
A fan-shaped molecule (2), carrying hydrogen-bonding amide groups in proximity to its polar aromatic core, self-assembles into a columnar liquid crystalline mesophase, which unprecedentedly possesses…
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Functionalization of Azapentabenzocorannulenes by Fivefold C-H Borylation and Cross-Coupling Arylation: Application to Columnar Liquid-Crystalline Materials.
TLDR
The present method expands the variety and utility of azapentabenzocorannulenes as promising π-conjugated cores by an iridium-catalyzed fivefold C-H borylation reaction that exhibits excellent regioselectivity.
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Electric-field-responsive handle for large-area orientation of discotic liquid-crystalline molecules in millimeter-thick films.
TLDR
It is reported that aromatic amides with branched paraffinic tails, when properly spaced from mesogenic discotic cores, serve as an E-field-responsive handle that enables large-area unidirectional orientation of columnarly assembled LC molecules with extended p-conjugated cores.
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