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Domino Ring Expansion: Regioselective Access to 9-Membered Lactones with a Fused Indole Unit from 2-Nitrophenyl-1,3-cyclohexanediones.
The domino anionic fragmentation of 2-nitrophenyl-1,3-cyclohexanediones containing an electrophilic appendage such as aldehyde and epoxide is disclosed and provides an original access to decorated 9-membered lactones with a fused indole unit. Expand
Nucleophilic-Addition-Initiated Ring Expansion and Selectivity in Anionic Fragmentation.
The expansion of rings into larger ones by a mechanism of anionic fragmentation is a potent tool for exploring new structural space in a concise manner. As the concept has been known and applied for… Expand
Study toward an Asymmetric and Catalytic Synthesis of Koumine
A synthetic study of koumine, a natural product with a densely functionalized and inspiring heterocyclic skeleton, was conducted by exploring a strategy of desymmetrization of 1,3-cyclohexanedione by… Expand