D. Dimitrovski

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The possibility that memory is related to the collective rotational energy levels of the molecules is considered. Treating the molecule as a quantum rotator, the probability of the ‘‘hidden-crossing’’ transitions between rotational states, induced by the external periodic electric field, is analyzed. It is found that this probability depends on frequency(More)
We present an ellipticity-resolved study of momentum distributions arising from strong-field ionization of helium. The influence of the ion potential on the departing electron is considered within a semiclassical model consisting of an initial tunneling step and subsequent classical propagation. We find that the momentum distribution can be explained by(More)
A nanosecond laser pulse confines the spatial orientation of naphthalene in 1D or 3D while a femtosecond kick pulse initiates rotation of the molecular plane around the fixed long axis. Time-dependent photoelectron angular distributions (PADs), resulting from ionization by an intense femtosecond probe pulse, exhibit pronounced changes as the molecular plane(More)
The 3D photoelectron momentum distributions created by the strong-field ionization of argon atoms and naphthalene molecules with intense, large ellipticity (∼0.7) femtosecond laser pulses are studied. The experiment reveals the presence of low-energy electrons for randomly oriented naphthalene, but not for argon. Our theory shows that the induced dipole(More)
We investigate ionization and excitation of H(1s) in the limit of very short electric field pulses, analytically and numerically and both in the limit of small and extremely large peak electric fields. We identify a process of recombination akin to Rabi flopping from the continuum and give an analytic expression for this process after a single-cycle(More)
We present combined experimental and theoretical results on strong-field ionization of oriented carbonyl sulfide molecules by circularly polarized laser pulses. The obtained molecular frame photoelectron angular distributions show pronounced asymmetries perpendicular to the direction of the molecular electric dipole moment. These findings are explained by a(More)
Naphthalene molecules are fixed in space by a laser field and rotated, in 2° steps, over 180°. For each orientation, they are ionized by an intense, circularly polarized femtosecond laser pulse, and the 2D projection of the photoelectron momentum distribution is recorded. The molecular-frame 3D momentum distribution is obtained by tomographic reconstruction(More)
We present a combined experimental and theoretical study on strong-field ionization of a three-dimensionallyoriented asymmetric top molecule, benzonitrile (C7H5N), by circularly polarized, nonresonant femtosecond laser pulses. Prior to the interaction with the strong field, the molecules are quantum-state selected using a deflector and three-dimensionally(More)
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